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We develop novel methodologies for the synthesis of novel supramolecular architectures. Our interest is mainly directed to the synthesis of supramolecular cages and to exploit their applications in molecular recognition and catalysis . Chirality, in term of sensing and study of novel chiroptical properties, is also something we are carried on. All prepared molecular architectures have in common the presence of tris(2-pyridylmethyl)amine (TPMA) metal complexes which, as mononuclear systems or as more complex architectures, are able to display interesting properties as catalyst or receptors.